Some random thoughts about tapewounds (I have the Rotosounds) versus flats:
Tapewounds feel like they have less tension than chromes to me.... but the bass neck says otherwise
Soundwise, I loved the tape wounds. More of an DB tone than the chromes. The chromes are definitely brighter and have more sustain.
I would have stuck with the tapes, but I have some hum issues, and need steel strings to ground the hum.