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I think that you will find that the same strings have varied tone qualities on different basses. So, IMHO, it pretty much depends both on the bass and the tone you seek.
FWIW, I've ran the full gamut of flatwound strings on multiple basses (and have 5x one gallon bags of strings to do it again if needed) - some basses like chromes, others like TI's/LaBella's/77's/Legends, Precision Flats, etc.
I'm using Chromes on one P and TI's on another. GHS Precision Flats are a bit too dark for me - but if I was looking for a "dark" string, that's where I'd go. LaBella's (IMHO) take too long to break in (but last almost forever) - though I do use a mix of LaBellas to get the feel/tension/gauge that I want on one bass. 77's weren't the tone I was looking for - neither were Pyramids.
However, Chromes have just a touch of treble that can be dialed down with the tone control - but the sound still cuts through. TI's however have great mids and lows and are lower tension.
Again IMHO, the quality/quantity of mids is where good flats shine. Pretty much all of them have various levels of initial brightness and solid lows after they are broken in. Each though has different flavors of mids that are either desirable or not.
Long story short, welcome to your tone search.
John
As always, the above is IMHO and YMMV.
I have to agree with @iiipopes with my preference being Fender 9050 flats in any gauge you like.None of the above. The purpose of a Seymour Duncan Quarter Pounder is to add girth, punch and articulation. For that I would use either Fender flats 45-100 or Ernie Ball flats (regular, not cobalt) to take advantage of the grind this pickup can deliver.
I used the RotoSound 77s almost exclusively for several years. I'm now using the Chromes 45 - 100 (set ECB81) on all my basses except fretless, which wear D'Addario black tapes.
Why the legends? This thread topic has me intrigued. Thinking about flats for my Spector. Have had 77’s on other bass’s but wound up with nickel round cores on those. Specter currently wears Swing 66I’ve tried Labellas, Fenders, and TI Flats.
Without a doubt, I would recommend DR Legends. No hesitation.
I like Chromes once they're well broken in, but my first choice would be LaBella 760FLs - 43-104 or 760FSs - 45-105. Of course YMMV.