I cant really speak from experience on power supply modifications on 200S models; all of my 200Ss are stock except for one I sacrificed for a project testing circuit mods. The 200S I normally use for gigging has stock caps that were reformed a couple of years ago and still performs great, and the rest of them, Im a little ashamed to admit, are pretty much just gathering dust in my shop.
Ive got 2000Ss with three different power supply configurations, one is SS rectified with an SDS cap board installed;
SDS Labs Mk3 Capacitor Board, with parts and instructions
One SS rectified with a German Authenticap KTL13;
Frag Jan zuerst- Ask Jan first: Roehren und mehr
And the control in this comparison, a stock tube rectified one that amazingly still specs near new.
They sound different, the 2000S switched to SS rectification around 1970 and the later amps (including the amps renamed 350B) are noticeably stronger than the earlier tube rectified models.
The SDS mod is the strongest and stiffest, particularly in low end response, although it still retains the same basic tonal character inherent to the 2000S IMO. The Authenticap amp sounds like a standard SS rectified 2000S, not too surprising since the values are the same as the OEM Mallory was, just rated at 550V+ rather than the underrated 525V can cap was.
The stock tube rectified amp is a little softer; with less juice and gets a little more Pappalardi at lower levels than the SS rectified amps.
Overall IMO the CE or Authenticap is the easiest to use. Also as Greg points out, particularly with contemporary wall voltages the original 525V can cap will be stressed beyond its design spec. Since the Authenticap retains the original cap values but increases the voltage rating to 550V+ for the foreseeable future I will probably use them for any vintage Sunn recap jobs. Call it "old tech", but I also recently restocked my supply of big old Sprauge 20uf 600V electrolytics...
All of the 2000Ss will get loud and clean, you need to push them pretty hard to get the super hairy 60s distortion like Pappalardi was noted for. I think Felix often actually used lower powered 200S amps dimed to attain that over the top fuzzy distortion, and the mudbucker equipped Gibsons contributed as well!
The SDS amp gets the most use. I use it as backup for the Reeves C225 that serves as my main gig amp; occasionally I use the 2000S and keep the Reeves in reserve, but the SDS 2000S goes out pretty much every time I play.