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Best flatwound for a Chris Squire tone?

Not a string thing, but I would say go ricken for a bass. That is his tone in a nut shell. The rotos are great, but you will never get his true tone in my opinion without a ricken. He also has a couple of custom made basses, one of which I think, though I might be wrong, is a warwick. When I saw them in 2000 for thr ladder tour he was playing it, but I never could find out what it wasm I searched for it, nothing. Then this year when I saw them, he was all ricken the whole time. Those rotos are great, but nothing beats his bass. But you will have to see what works for you.
 
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I was playing my Fender Jazz with DSR Black Beauties, and I got a "similar" tone by playing aggressive fingerstyle down by the bridge. It isn't a dead-on thing, but it was nice.

I was playing Roundabout, and it sounded pretty good. I tried it with a pick, too, but I'm just not skilled enough at that.

But any Fender Jazz or Rick with any roundwound should get you pretty darn close. I don't see the need to exactly duplicate anybody's tone.

Be yourself!
 
+1 on the RotoSound Swing Bass 66 steel rounds. I tried some on one of my Rics. The hype is real, there is nothing like them. Downside is they die really fast. I got about 2~3 weeks out of them before they sounded deader than a set of nickels. Even Bass Brites can't bring 'em back. So if you are committed, and have a healthy budget, go for it! Otherwise, get a set of DR Hi-Beams or Lo-Rider steels. About as close as you can get string-wise without breaking the bank.