Maybe try Ernie Ball Cobalt flats. Very full range string and they don't have the high end 'zing' that Chromes have. Supple under the fingers. Take the time to clean them before installation.
I second this. Haven't played them on a fretless, but I've been super happy with them. They give up a smidge of high end compared to rounds, but the overall tone is there, and they let me slide all I want (I bring some guitar approach to my bass playing).